Layered Double Hydroxide Coated by Carbon-Based Material for Environmental Dye Pollutant

Authors

  • Neza Rahayu Palapa Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Sriwijaya, Indralaya, 30862, Indonesia
  • Alfan Wijaya Graduate School of Enviroment, Universitas Sriwijaya, Palembang, 30139, Indonesia

DOI:

https://doi.org/10.26554/ijmr.20231311

Keywords:

Dye Adsorption, Water Treatments, LDH Modification , Carbon-Based Material

Abstract

We conducted this research to modify NiAl layered double hydroxide with several carbon-based materials, including cellulose, biochar and graphite. This material was successfully prepared by coprecipitation methods and was proven by XRD, SEM and FTIR characterization. Furthermore, we conducted the adsorption process and reusability to investigate their ability as water treatments. The dose effect on M.G. removal was investigated by the highest M.G. removal capacity using the CBC-NiAl LDHs composite, which was 100 mg. M.G. removal capacity was increased with an increase in contact time, and the saturation point was reached after 60 min for CC-NiAl and CGF-NiAl LDHs, which CBC-NiAl LDH increased and saturated after 100 min with high adsorption capacity. CC-NiAl, CBC-NiAl and CGF-NiAl LDHs composite have proved efficient, sustainable materials that maintain adsorption capability in each reusable cycle.

References

Alagha, O., M. S. Manzar, M. Zubair, I. Anil, N. D. Mu’azu, and A. Qureshi (2020). Magnetic Mg Fe/LDH Intercalated Activated Carbon Composites for Nitrate and Phosphate Removal from Wastewater: Insight into Behavior and Mechanisms. Nanomaterials, 10(7); 1361

Amin, M., A. Alazba, and M. Shafiq (2022). Ldh of NiZnFe and Its Composites with Carbon Nanotubes and Data-Palm Biochar with Efficient Adsorption Capacity for Rb5 Dye from Aqueous Solutions: Isotherm, Kinetic, and Thermodynamics Studies. Current Applied Physics, 40; 90–100

Barkhordari, S. and M. Yadollahi (2016). Carboxymethyl Cellulose Capsulated Layered Double Hydroxides/Drug Nanohybrids for Cephalexin Oral Delivery. Applied Clay Science, 121; 77–85

Chang, J. H., P. Sivasubramanian, C. D. Dong, and M. Kumar (2023). Study on Adsorption of Ammonium and Nitrate in Wastewater by Modified Biochar. Bioresource Technology Reports, 21; 101346

Chen, H., T. Liu, Y. Meng, Y. Cheng, J. Lu, and H. Wang (2020). Novel Graphene Oxide/Aminated Lignin Aerogels for Enhanced Adsorption of Malachite Green in Wastewater. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 603; 125281

Choong, C. E., K. T. Wong, S. B. Jang, P. Saravanan, C. Park, S.-H. Kim, B.-H. Jeon, J. Choi, Y. Yoon, and M. Jang (2021). Granular Mg-Fe Layered Double Hydroxide Prepared Using Dual Polymers: Insights into Synergistic Removal of As(III) and As(V). Journal of Hazardous Materials, 403; 123883

Hakim, Y. M., R. Vinsiah, and S. Fajri (2023). High Efficient of Ca/Al-Graphite for Removal of Direct Orange. Indonesian Journal of Material Research, 1(1); 15–22

Jaffari, Z. H., A. Abbas, S. M. Lam, S. Park, K. Chon, E. S. Kim, and K. H. Cho (2023). Machine Learning Approaches to Predict the Photocatalytic Performance of Bismuth Ferrite-Based Materials in the Removal of Malachite Green. Journal of Hazardous Materials, 442; 130031

Khajeh, R. T., S. Aber, and M. Zarei (2020). Comparison of NiCo2O4, CoNiAl-LDH, and CoNiAl-LDH@NiCo2O4 Performances as ORR Catalysts in MFC Cathode. Renewable Energy, 154; 1263-1271

Kundu, S. and M. K. Naskar (2021). Carbon-Layered Double Hydroxide Nanocomposite for Efficient Removal of Inorganic and Organic Based Water Contaminants–Unravelling the Adsorption Mechanism. Materials Advances, 2(11); 3600–3612

Li, S., L. Dong, Z. Wei, G. Sheng, K. Du, and B. Hu (2020). Adsorption and Mechanistic Study of the Invasive Plant-Derived Biochar Functionalized with CaAl-LDH for Eu(III) in Water. Journal of Environmental Sciences, 96; 127–137

Liu, J. C., B. Qi, and Y. F. Song (2020). Engineering Polyoxometalate-Intercalated Layered Double Hydroxides for Catalytic Applications. Dalton Transactions, 49(13); 3934–3941

Machrouhi, A., M. Khnifira, W. Boumya, M. Sadiq, M. Abdennouri, A. Elhalil, F. Mahjoubi, and N. Barka (2023). Experimental and Density Functional Theory Studies of Methyl Orange Adsorption on Ni-Al/LDH Intercalated Sodium Dodecyl Sulfate. Chemical Physics Impact, 6; 100214

Mourid, E. H., M. Lakraimi, L. Benaziz, E. H. Elkhattabi, and A. Legrouri (2019). Wastewater Treatment Test by Removal of the Sulfamethoxazole Antibiotic by a Calcined Layered Double Hydroxide. Applied Clay Science, 168; 87–95

Oktriyanti, M. M., N. R. Palapa, R. Mohadi, and A. Lesbani (2019). Modification Of Zn-Cr Layered Double Hydroxide With Keggin Ion [α-SiW12O40]4− As Cr(VI) Adsorbent. Indonesian Journal of Environmental Management and Sustainability, 3(3); 93–99

Palapa, N. R., P. M. S. B. N. Siregar, A. Wijaya, T. Taher, and A. Lesbani (2022). High Selectivity and Stability Structure of Layered Double Hydroxide-Biochar for Removal Cd(II). Bulletin of Chemical Reaction Engineering & Catalysis, 17(3); 520–532

Palapa, N. R., T. Taher, A. Wijaya, and A. Lesbani (2021). Modification of Cu/Cr Layered Double Hydroxide by Keggin Type Polyoxometalate As Adsorbent of Malachite Green from Aqueous Solution. Science and Technology Indonesia, 6(3); 209–217

Palapa, N. R., A. Wijaya, N. Ahmad, A. Amri, R. Mohadi, and A. Lesbani (2023a). Activated Hydrochar Prepared from Longan Fruit (Dimocarpus longan Lour.) Peel via Hydrothermal Carbonization-NaOH Activation for Cationic Dyes Removal. Science and Technology Indonesia, 8(3); 461–470

Palapa, N. R., A. Wijaya, P. M. S. B. N. Siregar, A. Amri, N. Ahmad, T. Taher, and A. Lesbani (2023b). Adsorption of Fe(II) by Layered Double Hydroxide Composite with Carbon-Based Material (Biochar and Graphite): Reusability and Thermodynamic Properties. Indonesian Journal of Chemistry, 23(1); 101–112

Poudel, M. B., M. Shin, and H. J. Kim (2022). Interface Engineering of MIL-88 Derived MnFe-LDH and MnFe2O3 on ThreeDimensional Carbon Nanofibers for the Efficient Adsorption of Cr(VI), Pb(II), and As(III) Ions. Separation and Purification Technology, 287; 120463

Qu, W., T. Yuan, G. Yin, S. Xu, Q. Zhang, and H. Su (2019). Effect of Properties of Activated Carbon on Malachite Green Adsorption. Fuel, 249; 45–53

Sadiq, A. C., N. Y. Rahim, and F. B. M. Suah (2020). Adsorption and Desorption of Malachite Green by Using Chitosan-Deep Eutectic Solvents Beads. International Journal of Biological Macromolecules, 164; 3965–3973

Sajid, M., S. M. S. Jillani, N. Baig, and K. Alhooshani (2022). Layered Double Hydroxide-Modified Membranes for Water Treatment: Recent Advances and Prospects. Chemosphere, 287; 132140

Salem, M. A., A. M. Khan, Y. K. Manea, and A. A. Wani (2022). Nano Chromium Embedded in f-CNT Supported CoBi-LDH Nanocomposites for Selective Adsorption of Pb2+ and Hazardous Organic Dyes. Chemosphere, 289; 133073

Sharma, J., S. Sharma, and V. Soni (2023). Toxicity of Malachite Green on Plants and Its Phytoremediation: A Review. Regional Studies in Marine Science, 62; 102911

Siregar, P. M. S. B. N., N. R. Palapa, A. Wijaya, E. S. Fitri, and A. Lesbani (2021). Structural Stability of Ni/Al Layered Double Hydroxide Supported on Graphite and Biochar toward Adsorption of Congo Red. Science and Technology Indonesia, 6(2); 85–95

Srivastava, S., R. Sinha, and D. Roy (2004). Toxicological Effects of Malachite Green. Aquatic Toxicology, 66(3); 319–329

Taher, T., Y. G. Wibowo, S. Maulana, N. R. Palapa, A. Rianjanu, and A. Lesbani (2023). Facile Synthesis of Biochar/layered Double Oxides Composite by One-Step Calcination for Enhanced Carbon Dioxide (CO2) Adsorption. Materials Letters, 338; 134068

Wang, J., X. Mei, L. Huang, Q. Zheng, Y. Qiao, K. Zang, S. Mao, R. Yang, Z. Zhang, Y. Gao, et al (2015). Synthesis of Layered Double Hydroxides/Graphene Oxide Nanocomposite As a Novel High-Temperature CO2 Adsorbent. Journal of Energy Chemistry, 24(2); 127–137

Zhang, D., M. Zhao, H. Zhang, M. Terrones, and Y. Wang (2023). A Novel Electro-Synthesis of Hierarchical Ni-Al LDH Nanostructures on 3D Carbon Nanotube Networks for Hybrid-Capacitors. Carbon, 201; 1081–1

Downloads

Published

2023-11-29

Issue

Section

Articles